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Inverse uncertainty characteristics of pollution source identification for river chemical spill incidents

Jiping Jiang, Feng Han, Yi Zheng, Nannan Wang, Yixing Yuan

《环境科学与工程前沿（英文）》 2018年 第12卷 第5期 doi: 10.1007/s11783-018-1081-4

摘要：

Uncertainty rules of pollution source inversion are revealed by stochastic analysis

A release load is most easily inversed and source locations own largest uncertainty

Instantaneous spill assumption has much less uncertainty than continuous spill

The estimated release locations and times negatively deviate from real values

The new findings improve monitoring network design and emergency response to spills

关键词： River chemical spills     Emergency response     Pollution source inversion     Inverse uncertainty analysis     Regional Sensitivity Analysis method (RSA)     Monte Carlo analysis toolbox (MCAT)    

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Applying chemical sedimentation process in drinking water treatment plant to address the emergent arsenicspills in water sources

Pengfei LIN,Xiaojian ZHANG,Hongwei YANG,Yong LI,Chao CHEN

《环境科学与工程前沿（英文）》 2015年 第9卷 第1期   页码 50-57 doi: 10.1007/s11783-014-0733-2

摘要： Arsenic (As) spills occurred more frequently and sometimes polluted water sources in recent years in China. It is as urgent need to develop emergency treatment technologies to address the arsenic threat for large-scale water treatment plants. In response, we developed a chemical sedimentation technology to remove arsenic contaminants for water treatment plants. Bench-scale experiments were conducted to investigate the efficiency of arsenic removal and the influencing factors of the chemical sedimentation treatment process. The influencing factors included the choice and dosage of coagulants, the valence of arsenic and pH value of solution. The As(V) contaminants can be almost completely removed by ferric or alum coagulants. The As(III) contaminants are more recalcitrant to chemical sedimentation, 75% for ferric coagulant and 40% for alum coagulant. The quantitative results of arsenic removal load by different ferric or alum coagulants were presented to help determine the parameters for arsenic treatment technology. The dominant mechanism for arsenic removal is static combination, or adsorption of negative arsenic species onto positive ferric hydroxide or alum hydroxide flocs. The efficiency of this treatment technology has also been demonstrated by a real production test in one water treatment plant with arsenic-rich source water and one emergency response. This technology was verified to be quick to set-up, easy to operate and highly efficient even for high concentration of arsenic.

关键词： Arsenic spill     chemical sedimentation     coagulation     drinking water     emergency treatment    

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Two-dimensional numerical and eco-toxicological modeling of chemical spills

Suiliang HUANG, Yafei JIA, Sam S. Y. WANG

《环境科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 178-185 doi: 10.1007/s11783-009-0020-9

摘要： The effects of chemical spills on aquatic non-target organisms were evaluated in this study. Based on a review of three types of current eco-toxicological models of chemicals, i.e., ACQUATOX model of the US-EPA, Hudson River Model of PCBs, and critical body residual (CBR) model and dynamic energy budget (DEBtox) model, this paper presents an uncoupled numerical eco-toxicological model. The transport and transformation of spilled chemicals were simulated by a chemical transport model (including flow and sediment transport), and the mortalities of an organism caused by the chemicals were simulated by the extended threshold damage model, separately. Due to extreme scarcity of data, this model was applied to two hypothetical cases of chemical spills happening upstream of a lake. Theoretical analysis and simulated results indicated that this model is capable of reasonably predicting the acute effects of chemical spills on aquatic ecosystems or organism killings.

关键词： chemical spills     acute effects     aquatic ecosystem     eco-toxicological modeling    

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chlorinated aromatics' structure on their adsorption characteristics on activated carbon to tackle chemicalspills in drinking water source

Pengfei LIN,Yuan ZHANG,Xiaojian ZHANG,Chao CHEN,Yuefeng XIE,Irwin H SUFFET

《环境科学与工程前沿（英文）》 2015年 第9卷 第1期   页码 138-146 doi: 10.1007/s11783-014-0725-2

摘要： This study focused on evaluating the efficiency of powdered activated carbon (PAC) adsorption process and tackling chlorobenzenes and chlorophenols spill in drinking water source. The adsorption kinetics and PAC’s capacities for five chlorobenzenes and three chlorophenols at drinking water contamination levels were studied in order to determine the influence of different functional groups on the adsorption behavior. The results showed that PAC adsorption could be used as an effective emergency drinking water treatment process to remove these compounds. The adsorption kinetics took 30 min to achieve nearly equilibrium and could be described by both pseudo first-order and pseudo second-order models. A mathematic relationship was developed between the pseudo first-order adsorption rate constant, k , and the solutes’ properties including lg , polarizability and molecular weight. The Freundlich isotherm equation could well describe the adsorption equilibrium behaviors of chlorinated aromatics with from 0.920 to 0.999. The H-bond donor/acceptor group, hydrophobicity, solubility and molecular volume were identified as important solute properties that affect the PAC adsorption capacity. These results could assist water professionals in removing chlorinated aromatics during emergency drinking water treatment.

关键词： chlorinated aromatics     adsorption     powdered activated carbon     kinetics     equilibrium    

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A 50-year sedimentary record of heavy metals and their chemical speciations in the Shuangtaizi River

Baolin LIU, Ke HU, Zhenglong JIANG, Fengge QU, Xin SU

《环境科学与工程前沿（英文）》 2011年 第5卷 第3期   页码 435-444 doi: 10.1007/s11783-011-0352-0

摘要： Two parallel sediment cores collected from tidal flat located in the Shuangtaizi River estuary were analyzed for heavy metal concentrations and chemical speciations. Based on the Cs activity profile, mean sedimentation rate at the sampling site during the past 50 years was estimated to be 1.3 cm·a . Correlation analyses show that almost all the metals are associated with each other, suggesting that these metals might be derived from same sources and/or affected by same geochemical processes. Influence of total organic carbon (TOC) content on the concentrations of Cr, Ni, Cu and Cd is evident. Silt and clay contents, instead of sand content, play an important role in the distribution of these metals. The dominant binding phases for most of the metals (except for Cd) are the residual. The relative decrease of the residual fraction of Cd and Pb in the upper 66 cm of the core is striking. The distribution of chemical fraction confirms that the residual fractions of these metals have a natural origin, while only the non-residual fractions of Cd and Pb increased upward the core due to pollution in the past five decades. Pollution assessment on these heavy metals based on Index of Geoaccumulation ( ) also demonstrates that most of the metals are unpolluted. The weak pollution as observed in the sediments is perhaps related to a local plant, the Kitag, which may have played a significant role in the biodegradation of these metals and the metal distribution in the estuary.

关键词： Shuangtaizi River estuary     sediment core     heavy metals     pollution    

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Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 53-62 doi: 10.1007/s11783-014-0728-z

摘要： Understanding the trends in PM levels is essential for formulating clean air plans. This paper analyzes PM data from various published sources for the years 2000 to 2010 in the Pearl River Delta Economic Zone (PRDEZ). The long-term variation in PM mass concentration is analyzed. Results show that PM , organic carbon (OC), elemental carbon (EC), and show a similar trend, increasing before 2005 and then decreasing slightly. The annual average PM concentration ranges from 49.1 μg·m in 2000 to 64.3 μg·m in 2010, with a peak of 84.1 μg·m in 2004. None of these 11 years meets the new National Ambient Air Quality standard (NAAQS) for PM (35 μg·m ). Overall average concentrations of OC, EC, and are 13.0, 6.5, and 11.8 μg·m , respectively. and respectively have concentrations of 1.5 μg·m and 2.9 μg·m in 2000 and 6.4 μg·m and 5.3 μg·m in 2010, with a statistically significant average annual trend of+ 0.2 μg·m ·yr and+ 0.1 μg·m ·yr . In certain geographic regions, OC and EC contribute most of the PM , while in other regions secondary water-soluble ions are more important. In general, OC and are the dominant components of PM , contributing 20.6% and 18.6%, respectively. These results provide, for the first time, a better understanding of the long-term PM characteristics and trends, on a species-by-species basis, in the PRDEZ. The results indicate that PM abatement needs to prioritize secondary species.

关键词： long-term trends     fine particulate matter     chemical components     Pearl River Delta Economic Zone (PRDEZ)    

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Sequence of the main geochemical controls on the Cu and Zn fractions in the Yangtze River estuarine sediments

Shou ZHAO,Dongxin WANG,Chenghong FENG,Ying WANG,Zhenyao SHEN

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 19-27 doi: 10.1007/s11783-014-0723-4

摘要： Metal speciation can provide sufficient information for environmental and geochemical researches. In this study, based on the speciation determination of Cu and Zn in the Yangtze Estuary sediments, roles of eight geochemical controls (i.e., total organic carbon (TOC), clay, Fe/Mn in five chemical fractions and salinity) are fully investigated and sequenced with correlation analysis (CA) and principal components analysis (PCA). Results show that TOC, clay and Fe/Mn oxides are key geochemical factors affecting the chemical speciation distributions of Cu and Zn in sediments, while the role of salinity appears to be more indirect effect. The influencing sequence generally follows the order: TOC>clay>Mn oxides>Fe oxides>salinity. Among the different fractions of Fe/Mn oxides, residual and total Fe content, and exchangeable and carbonate Mn exert the greatest influences, while exchangeable Fe and residual Mn show the poorest influences.

关键词： chemical speciation     geochemical factors     estuaries     sediments     correlation     salinity    

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TiO@palygorskite composite for the efficient remediation of oil spills via a dispersion-photodegradation

《环境科学与工程前沿（英文）》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1365-3

摘要：

• A novel and multi-functional clay-based oil spill remediation system was constructed.

关键词： Palygorskite     TiO2     Pickering emulsion     Oil spill     Dispersion     Photodegradation    

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Multi-scale evaluation of river health in Liao River Basin, China

Fei XU, Yanwei ZHAO, Zhifeng YANG, Yuan ZHANG

《环境科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 227-235 doi: 10.1007/s11783-010-0219-9

摘要： Previous studies on river health evaluation mainly focused on characterizations at a river-corridor scale and ignored the complex interactions between the river ecosystem and other components of the river basin. Based on the consideration of the interactions among rivers, associated river basin and habitats, an assessment framework with multi-scale indicators was developed. An index system divided among these three scales to characterize the health of river ecosystems in China’s Liao River Basin was established. Set pair analysis was applied to integrate the multi-scale indicators and determine the health classes. The evaluation results indicated that the rivers in the western and eastern zones of the Liao River were classified as sick, and rivers in the main stream of the Liao and Huntai rivers were classified as unhealthy. An excessive level of disturbances, such as large pollution loads and dense construction of water conservation projects within the river basin, were the main causes of the river health deterioration.

关键词： multi-scale characterization     river health evaluation     Liao River Basin     set pair analysis    

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Special issue on “Green chemical process and intensification”

《化学科学与工程前沿（英文）》 2022年 第16卷 第11期   页码 1533-1535 doi: 10.1007/s11705-022-2263-y

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Special Issue for the Future Chemical Engineering Scholars of Global Chinese Chemical Engineering Symposium

《化学科学与工程前沿（英文）》 2022年 第16卷 第6期   页码 775-776 doi: 10.1007/s11705-022-2172-0

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Insight of chemical environmental risk and its management from the vinyl chloride accident

《环境科学与工程前沿（英文）》 2023年 第17卷 第4期 doi: 10.1007/s11783-023-1652-x

摘要： The combustion of vinyl chloride (VC) after the train derailment accident in Ohio, USA in February, 2023 has caused widespread concern around the world. This paper tried to analyze several issues concerning the accident, including the appropriateness of the VC combustion in the emergency response in this accident, the meanings of so-called “controlled combustion”, the potential environmental risks caused by VC and combustion by-products, and follow-up work. In our view, this accident had surely caused environmental and health risks to some extent. Hence, a comprehensive environmental risk assessment is necessary, and then the site with risk should be comprehensively remediated, hazardous waste should be harmlessly treated as soon as possible. Finally, this accident suggests that further efforts should be taken to bridge the gap between chemical safety management and their environmental risk management.

关键词： Vinyl chloride     Combustion     Chemical safety management     Environmental risk     Emerging contaminants    

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Multiple Pollutants from Crop and Livestock Production in the Yangtze River: Status and Challenges

《农业科学与工程前沿（英文）》 doi: 10.15302/J-FASE-2023511

摘要：

● Cash crops and livestock production in Yangtze River Basin has grown rapidly.

关键词： Agriculture Green Development     crop production     livestock production     multi-pollutant models     multiple pollutants     Yangtze River Basin    

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Effects of sulfur on variations in the chemical speciation of heavy metals from fly ash glass

《环境科学与工程前沿（英文）》 2023年 第17卷 第10期 doi: 10.1007/s11783-023-1728-7

摘要：

● A higher sulfur content reduced the curing rate of Cr in glass.

关键词： Dechlorinated fly ash     SO3     Heavy metal     Chemical speciation     Glass solidification    

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Integrated river basin management in rapidly urbanizing areas: a case of Shenzhen, China

Lei LIU, Xiaoming MA

《环境科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 243-254 doi: 10.1007/s11783-010-0276-0

摘要： The rapid urbanization of China is causing a burden on their water resources and hindering their sustainable development. This paper analyzes effective methods to integrated river basin management (IRBM) using Longgang River basin of Shenzhen as an example, which is the city with the fastest rate of urbanization in China and even the whole world. Over the past 20 years, China has undergone a population boom due to the increase of immigrant workers and rapid development of labor-intensive industries, which led to the sharp increase of water consumption and sewage discharge. However, the construction of the water infrastructure is still lagging far behind the environmental and social development, with only 32.7% of sewage in the district being treated. Currently, every water quality indicator of the Longgang River basin was unable to meet the required corresponding environmental standards, which further aggravated the water shortages of the region. Thus, an analytical framework is proposed to address the IRBM of the study area. The problems with the current management system include the lack of decentralization in decision-making, lack of enforcement with redundant plans, weak management capacity, financial inadequacy, and a poor system of stakeholder participation. In light of the principles of IRBM and the situation of the region, corresponding measures are put forward, including an increase of power given to sub-district offices, fewer but more feasible plans, capacity building among stakeholders, a combination of planning and marketing for overcoming financial inadequacy, and profound reform in the public participation system. The framework and institutional suggestions could inform similar processes in other representative river basins.

关键词： integrated river basin management (IRBM) model     Longgang River basin     Shenzhen     decentralization     stakeholder participation    

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标题 作者 时间 类型 操作

Inverse uncertainty characteristics of pollution source identification for river chemical spill incidents

Jiping Jiang, Feng Han, Yi Zheng, Nannan Wang, Yixing Yuan

期刊论文

Applying chemical sedimentation process in drinking water treatment plant to address the emergent arsenicspills in water sources

Pengfei LIN,Xiaojian ZHANG,Hongwei YANG,Yong LI,Chao CHEN

期刊论文

Two-dimensional numerical and eco-toxicological modeling of chemical spills

Suiliang HUANG, Yafei JIA, Sam S. Y. WANG

期刊论文

chlorinated aromatics' structure on their adsorption characteristics on activated carbon to tackle chemicalspills in drinking water source

Pengfei LIN,Yuan ZHANG,Xiaojian ZHANG,Chao CHEN,Yuefeng XIE,Irwin H SUFFET

期刊论文

A 50-year sedimentary record of heavy metals and their chemical speciations in the Shuangtaizi River

Baolin LIU, Ke HU, Zhenglong JIANG, Fengge QU, Xin SU

期刊论文

Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

期刊论文

Sequence of the main geochemical controls on the Cu and Zn fractions in the Yangtze River estuarine sediments

Shou ZHAO,Dongxin WANG,Chenghong FENG,Ying WANG,Zhenyao SHEN

期刊论文

TiO@palygorskite composite for the efficient remediation of oil spills via a dispersion-photodegradation

期刊论文

Multi-scale evaluation of river health in Liao River Basin, China

Fei XU, Yanwei ZHAO, Zhifeng YANG, Yuan ZHANG

期刊论文

Special issue on “Green chemical process and intensification”

期刊论文

Special Issue for the Future Chemical Engineering Scholars of Global Chinese Chemical Engineering Symposium

期刊论文

Insight of chemical environmental risk and its management from the vinyl chloride accident

期刊论文

Multiple Pollutants from Crop and Livestock Production in the Yangtze River: Status and Challenges

期刊论文

Effects of sulfur on variations in the chemical speciation of heavy metals from fly ash glass

期刊论文

Integrated river basin management in rapidly urbanizing areas: a case of Shenzhen, China

Lei LIU, Xiaoming MA

期刊论文